Green Li+- and Er3+-doped poly(ε-caprolactone)/siloxane biohybrid electrolytes for smart electrochromic windows
Identifieur interne : 000119 ( Main/Repository ); précédent : 000118; suivant : 000120Green Li+- and Er3+-doped poly(ε-caprolactone)/siloxane biohybrid electrolytes for smart electrochromic windows
Auteurs : RBID : Pascal:14-0084068Descripteurs français
- Pascal (Inist)
- Matériau dopé, Electrolyte, Vitrage, Matériau intelligent, Electrochromisme, Dispositif électrochromique, Procédé sol gel, Protection environnement, Impact environnement, Prototype, Addition étain, Couche ITO, Commutation, Réversibilité, Evaluation performance, Circuit ouvert, Facteur transmission, Densité optique, Rendement énergétique, Siloxane, Polymère réticulé, Lithium, Erbium, Verre, Oxyde d'indium, Oxyde de tungstène, Matériau conducteur, Matériau transparent, ITO, WO3.
- Wicri :
- concept : Prototype, Rendement énergétique, Verre.
English descriptors
- KwdEn :
- Conducting material, Crosslinked polymer, Doped materials, Electrochromic device, Electrochromism, Electrolyte, Energetic efficiency, Environment impact, Environmental protection, Erbium, Glass, ITO layers, Indium oxide, Lithium, Open circuit, Optical density, Performance evaluation, Prototype, Reversibility, Siloxanes, Smart materials, Sol gel process, Switching, Tin addition, Transmittance, Transparent material, Tungsten oxide, Window glazing.
Abstract
Novel electrolytes composed of a sol-gel derived di-urethane cross-linked poly(ε-caprolactone) (d-PCL (530))/siloxane (where 530 is the average molecular weight in g mol-1) biohybrid network doped with a 50:50 molar mixture of lithium and erbium triflates were prepared in the light of the "mixed cation effect". These environmentally friendly electrolytes, which are multi-wavelength emitters from the UV/ VIS to the NIR spectral regions, are attractive candidates for electrochromic devices. Prototype devices based on a glass/ITO/WO3/electrolyte/ITO/glass layered configuration exhibited fast switching speed, high electrochromic reversibility and cyclic stability, along with good coloration efficiency and open circuit memory. The visible average transmittance variation and the optical density change attained were 41.6% and 0.39, respectively. The combined use of these electrolytes with transparent conducting oxides in the VIS and NIR spectral regions opens exciting new prospects for the fabrication of electrochromic windows exhibiting NIR emission and improved performance in terms of energy efficiency in buildings. In addition, these electrolytes offer new possibilities for the production of dual light emitting and electrochromic windows.
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Pascal:14-0084068Le document en format XML
<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Green Li<sup>+</sup>- and Er<sup>3+</sup>-doped poly(ε-caprolactone)/siloxane biohybrid electrolytes for smart electrochromic windows</title><author><name sortKey="Fernandes, M" uniqKey="Fernandes M">M. Fernandes</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Chemistry Department and CQ-VR, University of Trás-os-Montes e Alto Douro</s1><s2>5000-801 Vila Real</s2><s3>PRT</s3><sZ>1 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>5000-801 Vila Real</wicri:noRegion></affiliation></author><author><name sortKey="Freitas, V T" uniqKey="Freitas V">V. T. Freitas</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Physics Department and CICECO, University of Aveiro</s1><s2>3810-193 Aveiro</s2><s3>PRT</s3><sZ>2 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Pereira, S" uniqKey="Pereira S">S. Pereira</name><affiliation wicri:level="1"><inist:fA14 i1="03"><s1>CENIMAT/13N, Departamento de Ciência dos Materiais, Faculdade de Ciências e Tecnologia, FCT, Universidade Nova de Lisboa and CEMOP-UNINOVA</s1><s2>2829-516 Caparica</s2><s3>PRT</s3><sZ>3 aut.</sZ><sZ>4 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>2829-516 Caparica</wicri:noRegion></affiliation></author><author><name sortKey="Fortunato, E" uniqKey="Fortunato E">E. Fortunato</name><affiliation wicri:level="1"><inist:fA14 i1="03"><s1>CENIMAT/13N, Departamento de Ciência dos Materiais, Faculdade de Ciências e Tecnologia, FCT, Universidade Nova de Lisboa and CEMOP-UNINOVA</s1><s2>2829-516 Caparica</s2><s3>PRT</s3><sZ>3 aut.</sZ><sZ>4 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>2829-516 Caparica</wicri:noRegion></affiliation></author><author><name sortKey="Ferreira, R A S" uniqKey="Ferreira R">R. A. S. Ferreira</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Physics Department and CICECO, University of Aveiro</s1><s2>3810-193 Aveiro</s2><s3>PRT</s3><sZ>2 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Carlos, L D" uniqKey="Carlos L">L. D. Carlos</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Physics Department and CICECO, University of Aveiro</s1><s2>3810-193 Aveiro</s2><s3>PRT</s3><sZ>2 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Rego, R" uniqKey="Rego R">R. Rego</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Chemistry Department and CQ-VR, University of Trás-os-Montes e Alto Douro</s1><s2>5000-801 Vila Real</s2><s3>PRT</s3><sZ>1 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>5000-801 Vila Real</wicri:noRegion></affiliation></author><author><name sortKey="De Zea Bermudez, V" uniqKey="De Zea Bermudez V">V. De Zea Bermudez</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Chemistry Department and CQ-VR, University of Trás-os-Montes e Alto Douro</s1><s2>5000-801 Vila Real</s2><s3>PRT</s3><sZ>1 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ></inist:fA14><country>Portugal</country><wicri:noRegion>5000-801 Vila Real</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="inist">14-0084068</idno><date when="2014">2014</date><idno type="stanalyst">PASCAL 14-0084068 INIST</idno><idno type="RBID">Pascal:14-0084068</idno><idno type="wicri:Area/Main/Corpus">000096</idno><idno type="wicri:Area/Main/Repository">000119</idno></publicationStmt><seriesStmt><idno type="ISSN">0927-0248</idno><title level="j" type="abbreviated">Sol. energy mater. sol. cells</title><title level="j" type="main">Solar energy materials and solar cells</title></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Conducting material</term><term>Crosslinked polymer</term><term>Doped materials</term><term>Electrochromic device</term><term>Electrochromism</term><term>Electrolyte</term><term>Energetic efficiency</term><term>Environment impact</term><term>Environmental protection</term><term>Erbium</term><term>Glass</term><term>ITO layers</term><term>Indium oxide</term><term>Lithium</term><term>Open circuit</term><term>Optical density</term><term>Performance evaluation</term><term>Prototype</term><term>Reversibility</term><term>Siloxanes</term><term>Smart materials</term><term>Sol gel process</term><term>Switching</term><term>Tin addition</term><term>Transmittance</term><term>Transparent material</term><term>Tungsten oxide</term><term>Window glazing</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Matériau dopé</term><term>Electrolyte</term><term>Vitrage</term><term>Matériau intelligent</term><term>Electrochromisme</term><term>Dispositif électrochromique</term><term>Procédé sol gel</term><term>Protection environnement</term><term>Impact environnement</term><term>Prototype</term><term>Addition étain</term><term>Couche ITO</term><term>Commutation</term><term>Réversibilité</term><term>Evaluation performance</term><term>Circuit ouvert</term><term>Facteur transmission</term><term>Densité optique</term><term>Rendement énergétique</term><term>Siloxane</term><term>Polymère réticulé</term><term>Lithium</term><term>Erbium</term><term>Verre</term><term>Oxyde d'indium</term><term>Oxyde de tungstène</term><term>Matériau conducteur</term><term>Matériau transparent</term><term>ITO</term><term>WO3</term></keywords><keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Prototype</term><term>Rendement énergétique</term><term>Verre</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Novel electrolytes composed of a sol-gel derived di-urethane cross-linked poly(ε-caprolactone) (d-PCL (530))/siloxane (where 530 is the average molecular weight in g mol<sup>-1</sup>) biohybrid network doped with a 50:50 molar mixture of lithium and erbium triflates were prepared in the light of the "mixed cation effect". These environmentally friendly electrolytes, which are multi-wavelength emitters from the UV/ VIS to the NIR spectral regions, are attractive candidates for electrochromic devices. Prototype devices based on a glass/ITO/WO<sub>3</sub>/electrolyte/ITO/glass layered configuration exhibited fast switching speed, high electrochromic reversibility and cyclic stability, along with good coloration efficiency and open circuit memory. The visible average transmittance variation and the optical density change attained were 41.6% and 0.39, respectively. The combined use of these electrolytes with transparent conducting oxides in the VIS and NIR spectral regions opens exciting new prospects for the fabrication of electrochromic windows exhibiting NIR emission and improved performance in terms of energy efficiency in buildings. In addition, these electrolytes offer new possibilities for the production of dual light emitting and electrochromic windows.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0927-0248</s0></fA01><fA03 i2="1"><s0>Sol. energy mater. sol. cells</s0></fA03><fA05><s2>123</s2></fA05><fA08 i1="01" i2="1" l="ENG"><s1>Green Li<sup>+</sup>- and Er<sup>3+</sup>-doped poly(ε-caprolactone)/siloxane biohybrid electrolytes for smart electrochromic windows</s1></fA08><fA11 i1="01" i2="1"><s1>FERNANDES (M.)</s1></fA11><fA11 i1="02" i2="1"><s1>FREITAS (V. T.)</s1></fA11><fA11 i1="03" i2="1"><s1>PEREIRA (S.)</s1></fA11><fA11 i1="04" i2="1"><s1>FORTUNATO (E.)</s1></fA11><fA11 i1="05" i2="1"><s1>FERREIRA (R. A. S.)</s1></fA11><fA11 i1="06" i2="1"><s1>CARLOS (L. D.)</s1></fA11><fA11 i1="07" i2="1"><s1>REGO (R.)</s1></fA11><fA11 i1="08" i2="1"><s1>DE ZEA BERMUDEZ (V.)</s1></fA11><fA14 i1="01"><s1>Chemistry Department and CQ-VR, University of Trás-os-Montes e Alto Douro</s1><s2>5000-801 Vila Real</s2><s3>PRT</s3><sZ>1 aut.</sZ><sZ>7 aut.</sZ><sZ>8 aut.</sZ></fA14><fA14 i1="02"><s1>Physics Department and CICECO, University of Aveiro</s1><s2>3810-193 Aveiro</s2><s3>PRT</s3><sZ>2 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></fA14><fA14 i1="03"><s1>CENIMAT/13N, Departamento de Ciência dos Materiais, Faculdade de Ciências e Tecnologia, FCT, Universidade Nova de Lisboa and CEMOP-UNINOVA</s1><s2>2829-516 Caparica</s2><s3>PRT</s3><sZ>3 aut.</sZ><sZ>4 aut.</sZ></fA14><fA20><s1>203-210</s1></fA20><fA21><s1>2014</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>18016</s2><s5>354000506140400270</s5></fA43><fA44><s0>0000</s0><s1>© 2014 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>36 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>14-0084068</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Solar energy materials and solar cells</s0></fA64><fA66 i1="01"><s0>NLD</s0></fA66><fC01 i1="01" l="ENG"><s0>Novel electrolytes composed of a sol-gel derived di-urethane cross-linked poly(ε-caprolactone) (d-PCL (530))/siloxane (where 530 is the average molecular weight in g mol<sup>-1</sup>) biohybrid network doped with a 50:50 molar mixture of lithium and erbium triflates were prepared in the light of the "mixed cation effect". These environmentally friendly electrolytes, which are multi-wavelength emitters from the UV/ VIS to the NIR spectral regions, are attractive candidates for electrochromic devices. Prototype devices based on a glass/ITO/WO<sub>3</sub>/electrolyte/ITO/glass layered configuration exhibited fast switching speed, high electrochromic reversibility and cyclic stability, along with good coloration efficiency and open circuit memory. The visible average transmittance variation and the optical density change attained were 41.6% and 0.39, respectively. The combined use of these electrolytes with transparent conducting oxides in the VIS and NIR spectral regions opens exciting new prospects for the fabrication of electrochromic windows exhibiting NIR emission and improved performance in terms of energy efficiency in buildings. In addition, these electrolytes offer new possibilities for the production of dual light emitting and electrochromic windows.</s0></fC01><fC02 i1="01" i2="X"><s0>001D06C02F</s0></fC02><fC02 i1="02" i2="X"><s0>230</s0></fC02><fC03 i1="01" i2="3" l="FRE"><s0>Matériau dopé</s0><s5>01</s5></fC03><fC03 i1="01" i2="3" l="ENG"><s0>Doped materials</s0><s5>01</s5></fC03><fC03 i1="02" i2="X" l="FRE"><s0>Electrolyte</s0><s5>02</s5></fC03><fC03 i1="02" i2="X" l="ENG"><s0>Electrolyte</s0><s5>02</s5></fC03><fC03 i1="02" i2="X" l="SPA"><s0>Electrólito</s0><s5>02</s5></fC03><fC03 i1="03" i2="X" l="FRE"><s0>Vitrage</s0><s5>03</s5></fC03><fC03 i1="03" i2="X" l="ENG"><s0>Window glazing</s0><s5>03</s5></fC03><fC03 i1="03" i2="X" l="SPA"><s0>Encristalado</s0><s5>03</s5></fC03><fC03 i1="04" i2="3" l="FRE"><s0>Matériau intelligent</s0><s5>04</s5></fC03><fC03 i1="04" i2="3" l="ENG"><s0>Smart materials</s0><s5>04</s5></fC03><fC03 i1="05" i2="X" l="FRE"><s0>Electrochromisme</s0><s5>05</s5></fC03><fC03 i1="05" 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l="SPA"><s0>Impacto medio ambiente</s0><s5>09</s5></fC03><fC03 i1="10" i2="X" l="FRE"><s0>Prototype</s0><s5>10</s5></fC03><fC03 i1="10" i2="X" l="ENG"><s0>Prototype</s0><s5>10</s5></fC03><fC03 i1="10" i2="X" l="SPA"><s0>Prototipo</s0><s5>10</s5></fC03><fC03 i1="11" i2="X" l="FRE"><s0>Addition étain</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="ENG"><s0>Tin addition</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="SPA"><s0>Adición estaño</s0><s5>11</s5></fC03><fC03 i1="12" i2="3" l="FRE"><s0>Couche ITO</s0><s5>12</s5></fC03><fC03 i1="12" i2="3" l="ENG"><s0>ITO layers</s0><s5>12</s5></fC03><fC03 i1="13" i2="X" l="FRE"><s0>Commutation</s0><s5>13</s5></fC03><fC03 i1="13" i2="X" l="ENG"><s0>Switching</s0><s5>13</s5></fC03><fC03 i1="13" i2="X" l="SPA"><s0>Conmutación</s0><s5>13</s5></fC03><fC03 i1="14" i2="X" l="FRE"><s0>Réversibilité</s0><s5>14</s5></fC03><fC03 i1="14" i2="X" l="ENG"><s0>Reversibility</s0><s5>14</s5></fC03><fC03 i1="14" i2="X" 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l="SPA"><s0>Erbio</s0><s2>NC</s2><s5>25</s5></fC03><fC03 i1="24" i2="X" l="FRE"><s0>Verre</s0><s5>26</s5></fC03><fC03 i1="24" i2="X" l="ENG"><s0>Glass</s0><s5>26</s5></fC03><fC03 i1="24" i2="X" l="SPA"><s0>Vidrio</s0><s5>26</s5></fC03><fC03 i1="25" i2="X" l="FRE"><s0>Oxyde d'indium</s0><s5>27</s5></fC03><fC03 i1="25" i2="X" l="ENG"><s0>Indium oxide</s0><s5>27</s5></fC03><fC03 i1="25" i2="X" l="SPA"><s0>Indio óxido</s0><s5>27</s5></fC03><fC03 i1="26" i2="X" l="FRE"><s0>Oxyde de tungstène</s0><s5>28</s5></fC03><fC03 i1="26" i2="X" l="ENG"><s0>Tungsten oxide</s0><s5>28</s5></fC03><fC03 i1="26" i2="X" l="SPA"><s0>Wolframio óxido</s0><s5>28</s5></fC03><fC03 i1="27" i2="X" l="FRE"><s0>Matériau conducteur</s0><s5>29</s5></fC03><fC03 i1="27" i2="X" l="ENG"><s0>Conducting material</s0><s5>29</s5></fC03><fC03 i1="27" i2="X" l="SPA"><s0>Material conductor</s0><s5>29</s5></fC03><fC03 i1="28" i2="X" l="FRE"><s0>Matériau transparent</s0><s5>30</s5></fC03><fC03 i1="28" i2="X" l="ENG"><s0>Transparent material</s0><s5>30</s5></fC03><fC03 i1="28" i2="X" l="SPA"><s0>Material transparente</s0><s5>30</s5></fC03><fC03 i1="29" i2="X" l="FRE"><s0>ITO</s0><s4>INC</s4><s5>82</s5></fC03><fC03 i1="30" i2="X" l="FRE"><s0>WO3</s0><s4>INC</s4><s5>83</s5></fC03><fN21><s1>111</s1></fN21><fN44 i1="01"><s1>OTO</s1></fN44><fN82><s1>OTO</s1></fN82></pA></standard></inist></record>Pour manipuler ce document sous Unix (Dilib)
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